<abstract xmlns="http://www.w3.org/1999/xhtml">The main objective of 235U irradiation is to obtain the 99mTc isotope, which is widely used in the domain of medical diagnostics. The decisive factor determining its availability, despite its short lifetime, is a reaction of radioactive decay of 99Mo into 99mTc. One of the possible sources of molybdenum can be achieved in course of the 235U fission reaction. The paper presents activities and the calculation results obtained upon the feasibility study on irradiation of 235U targets for production of 99Mo in the MARIA research reactor. Neutronic calculations and analyses were performed to estimate the fission products activity for uranium plates irradiated in the reactor. Results of dummy targets irradiation as well as irradiation uranium plates have been presented. The new technology obtaining 99Mo is based on irradiation of high-enriched uranium plates in standard reactor fuel channel and calculation of the current fission power generation. Measurements of temperatures and the coolant flow in the molybdenum installation carried out in reactor SAREMA system give online information about the current fission power generated in uranium targets. The corrective factors were taken into account as the heat generation from gamma radiation from neighbouring fuel elements as well as heat exchange between channels and the reactor pool. The factors were determined by calibration measurements conducted with aluminium mock-up of uranium plates. Calculations of fuel channel by means of REBUS code with fine mesh structure and libraries calculated by means of WIMS-ANL code were performed.</abstract>

The main objective of 235U irradiation is to obtain the 99mTc isotope, which is widely used in the domain of medical diagnostics. The decisive factor determining its availability, despite its short lifetime, is a reaction of radioactive decay of 99Mo into 99mTc. One of the possible sources of molybdenum can be achieved in course of the 235U fission reaction. The paper presents activities and the calculation results obtained upon the feasibility study on irradiation of 235U targets for production of 99Mo in the MARIA research reactor. Neutronic calculations and analyses were performed to estimate the fission products activity for uranium plates irradiated in the reactor. Results of dummy targets irradiation as well as irradiation uranium plates have been presented. The new technology obtaining 99Mo is based on irradiation of high-enriched uranium plates in standard reactor fuel channel and calculation of the current fission power generation. Measurements of temperatures and the coolant flow in the molybdenum installation carried out in reactor SAREMA system give online information about the current fission power generated in uranium targets. The corrective factors were taken into account as the heat generation from gamma radiation from neighbouring fuel elements as well as heat exchange between channels and the reactor pool. The factors were determined by calibration measurements conducted with aluminium mock-up of uranium plates. Calculations of fuel channel by means of REBUS code with fine mesh structure and libraries calculated by means of WIMS-ANL code were performed.

Production of Fission Product 99Mo using High-Enriched Uranium Plates in Polish Nuclear Research Reactor MARIA: Technology and Neutronic Analysis

Nuclear Energy Department, National Centre for Nuclear Research, 7 Andrzeja Sołtana Str., 05-400 Otwock/Świerk, Poland, Tel: +48 22 718 0077

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Production of Fission Product Mo using High-Enriched Uranium Plates in Polish Nuclear Research Reactor MARIA: Technology and Neutronic Analysis

The main objective of 235U irradiation is to obtain the 99mTc isotope, which is widely used in the domain of medical diagnostics. The decisive factor...

Production of Fission Product ⁹⁹Mo using High-Enriched Uranium Plates in Polish Nuclear Research Reactor MARIA: Technology and Neutronic Analysis

Article Category: Original Paper

Online veröffentlicht: 08. Juli 2014

Seitenbereich: 43 - 52

Eingereicht: 03. Okt. 2013

Akzeptiert: 28. Apr. 2014

DOI: https://doi.org/10.2478/nuka-2014-0009

Schlüsselwörter
fission products, Mo production, neutronic calculations, research reactor

© 2014 Janusz Jaroszewicz et. al.

This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 3.0 License.

Production of Fission Product 99Mo using High-Enriched Uranium Plates in Polish Nuclear Research Reactor MARIA: Technology and Neutronic Analysis

Article Category: Original Paper

Online veröffentlicht: 08. Juli 2014

Seitenbereich: 43 - 52

Eingereicht: 03. Okt. 2013

Akzeptiert: 28. Apr. 2014

DOI: https://doi.org/10.2478/nuka-2014-0009

Schlüsselwörterfission products, Mo production, neutronic calculations, research reactor

© 2014 Janusz Jaroszewicz et. al.

This work is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 3.0 License.

Production of Fission Product ⁹⁹Mo using High-Enriched Uranium Plates in Polish Nuclear Research Reactor MARIA: Technology and Neutronic Analysis

Schlüsselwörter
fission products, Mo production, neutronic calculations, research reactor