Fractions of heavy metals in soil after the application of municipal sewage sludge, peat, and furnace ash / Frakcje metali ciężkich w glebie po zastosowaniu komunalnego osadu ściekowego, popiołu paleniskowego i torfu

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Abstract

The effect of addition of different materials, i.e. sludge, ash and peat, as well as different doses of mixtures of ash and sludge and ash peat, on the total content of heavy metals (Cr, Zn, Pb, Cu, Cd, Ni) and their fractions was studied. Application of municipal sewage sludge, ash-sludge and ash-peat mixtures in the experiment caused a gradual increase in the content of studied heavy metals in soil. The ash was characterized by a low content of heavy metals as compared to municipal sewage sludge. After application of peat and its mixtures with ash a decrease of content of heavy metals was observed, and when the peat was used alone the greatest increase in the organic C content in the substrate could be seen. Distribution of heavy metals in the fractions separated in different combinations shows large variations, depending on the tested metal and the studied variant. Chromium, zinc, lead, and cadmium have been accumulated mainly in the residual fraction (FV), and most of the copper and nickel have been specifically bound with organic matter (FIV). It has been found that the alkaline materials application to the soil decreased the solubility of most heavy metals, which results in a limitation of their uptake by plants. Chromium and copper were an exception, since their solubility increased with the alkalinity of the substrate. An exception was chromium and copper, which solubility increased with the alkalinity of the substrate.

Al-Ani H., Oh E, Chai G., 2014. GIS-based examination of peats and soils in Surfers Paradise, Australia. Soil Science Annual, 65(1): 29-38.

Antonkiewicz J., 2007. Wp³yw ró¿nych mieszanin popio³owoosadowych i popio³owo-torfowych na plon i zawartooeæ pierwiastków w mieszance traw z komonic¹ zwyczajn¹. Czeoeæ II Metale ciê¿kie. (The influence of various ash-and-sludge and ash-and-peat mixtures on yield and elements content in grass birdsfoot-trefoil mixture. Part II. Heavy metals). Zeszyty Problemowe Postêpów Nauk Rolniczych - Advances of Agricultural Sciences Problem Issues, 520: 265-278.

Antonkiewicz J., 2008. Wp³yw komunalnego osadu oeciekowego, popio³u paleniskowego, torfu i ich mieszanin na w³aoeciwooeci fizykochemiczne oraz zawartooeæ metali ciê¿kich w glebie. (Influence of municipal sewage sludge incineration ash, peat and their mixtures on physicochemical properties and the heavy metals content in soil). Roczniki Gleboznawcze - Soil Science Annual, 59(1): 18-28.

Antonkiewicz J., 2011. Ocena biodostêpnooeci metali ciê¿kich w odpadach zastosowanych do przyrodniczej rekultywacji sk³adowiska odpadów niebezpiecznych. (Assessment of bioavailability of heavy metals in wastes used for biological reclamation of hazardous waste landfill). Zeszyty Naukowe Uniwersytetu Rolniczego w Krakowie, Nr 484, Seria Rozprawy 358, ss. 119 - Scientific Papers of the University of Agriculture in Krakow, No 481, Series Dissertation 358, 119 pp.

Aţýk B.B., Katkat A.V., 2010. Evaluation of wastewater sludge for possible agricultural use. Environmental Engineering and Management Journal, 10(6): 819-826.

Chang C-Y, Wang C-F, Mui D.T., Chiang H-L., 2009. Application of methods (sequential extraction procedures and highpressure digestion method) to fly ash particles to determine the element constituents: A case study for BCR 176. Journal of Hazardous Materials, 163: 578-587.

Dąbrowska L., Rosiñska A., Janosz-Rajczyk M., 2011. Heavy metals and PCBs in sewage sludge during thermophilic digestion process. Archives of Environmental Protection, 37(3): 3-13.

Gworek B., Mocek A., Kondzielski I., 2006. Speciation of copper in industrially polluted soils - a comparison of two sequential extraction methods. Polish Journal of Environmental Studies, 15(2a): 295-303.

Hanani M.N., Fauziah I.C., Samsuri A.W., Zauyah S., 2010. Formulation of Coal Fly Ash and Sewage Sludge Mixtures to Reduce Impacts on the Environment When Used as Soil Ameliorant for Acidic Tropical Soils. Malaysian Journal of Soil Science, 14: 53-70.

Hose G.C., Van den Brink P.J., 2004. Confirming the Species- Sensitivity Distribution Concept for Endosulfan Using Laboratory, Mesocosm, and Field Data. Archives of Environmental Contamination and Toxicology, 47: 511-520. DOI: 10.1007/s00244-003-3212-5.

Kabata-Pendias A., Piotrowska M., Motowicka-Terelak T., Maliszewska- Kordybach T., Filipiak K., Krakowiak A., Pietruch C., 1995. Podstawy oceny chemicznego zanieczyszczenia gleb - metale ciê¿kie, siarka i WWA. (Basis for the assessment of chemical contamination of soil - heavy metals, sulfur and PAHs). Pañstwowa Inspekcja Ochrony OErodowiska. Biblioteka Monitoringu OErodowiska - State Inspectorate for Environmental Protection. Library of Environmental Monitoring, Warsaw, pp. 41.

Kalembkiewicz J., Soèo E., 2004. Sequential extraction of Cr, Fe, Co, and Ni from industrial ash. Ecological Chemistry and Engineering, 11 (4-5): 347-352.

Legret M., 1993. Speciation of heavy metals in sewage sludge and sludge-amended soil. International Journal of Environmental Analytical Chemistry, 51: 161-166.

Legret M., Diver L and Juste C., 1988. Movement and speciation of heavy metals in a soil amended with sewage sludge containing large amount of cadmium and nickel. Water Research, 22(8): 953-969.

Papadimitriou C.A., Haritou I., Samaras P., Zouboulis A.I., 2008. Evaluation of leaching and ecotoxicological properties of sewage sludge-fly ash mixtures. Environmental Research, 106: 340-348.

Qin F., Wen B., Shan X-Q, Xie Y-N, Liu T., Zhang S-Z., Khan S.U., 2006. Mechanisms of competitive adsorption of Pb, Cu, and Cd on peat. Environmental Pollution, 144: 669-680.

Regulation, 2010. Regulation of the Minister of the Natural Environment on municipal sewage sludge dated 13 July 2010. Journal of Laws of Poland, No 137, Item 924.

Rosik-Dulewska C., G³owala K., Karwaczyñska U., Robak J., 2008. Elution of heavy metals from granulates produced from municipal sewage deposits and fly-ash of hard and brown coal in the aspect of recycling for fertilization purposes, Archives of Environmental Protection, 34(2): 63-72.

Samaras P., Papadimitriou C.A., Haritou I., Zouboulis A.I., 2008. Investigation of sewage sludge stabilization potential by the addition of fly ash and lime. Journal of Hazardous Materials, 154: 1052-1059.

Shrivastava S.K., Banerje D.K., 2004. Speciation of metals in sewage sludge and sludge-amended soils. Water, Air, and Soil Pollution, 152: 219-232.

Sienkiewicz S., Czarnecka M.H., 2012. Content of available Cu, Zn and Mn in soil amended with municipal sewage sludge. Journal of Elementology, 17(4): 649-657. DOI: 10.5601/jelem. 2012.17.4.08.

Sočo E., Kalembkiewicz J., 2007. Investigations of sequential leaching behaviour of Cu and Zn from coal fly ash and their mobility in environmental conditions. Journal of Hazardous Materials, 145: 482-487.

Syrovetnik K., Malmström M.E., Neretnieks I., 2008. Modelling retention of heavy metals in the Oostriku peat bog, Estonia: Comparison of predicted and observed results. Applied Geochemistry, 23: 1498-1512.

Systematyka gleb Polski (Classification of Polish Soils), 2011. Roczniki Gleboznawcze - Soil Science Annual, 62(3): 1-193.

Tessier A., Campbell P.G.C., Bisson M., 1979. Sequential extraction procedure for the speciation of particulate trace metals. Analytical Chemistry, 51(7): 844-851.

Weidong L., Ming L., Weifeng L., Haifeng L., 2010. Study on the ash fusion temperatures of coal and sewage sludge mixtures. Fuel, 89: 1566-1572.

Xua J-Q., Yua R-L., Dongb X-Y., Hua G-R., Shanga X-S., Wangc Q., Li H-W., 2012. Effects of municipal sewage sludge stabilized by fly ash on the growth of Manilagrass and transfer of heavy metals. Journal of Hazardous Materials, 217-218: 58-66.

Zhang F.-S., Yamasaki S.-I, Nanzyo M., Kimura K., 2001. Evaluation of cadmium and other metal losses from various municipal wastes during incineration disposal. Environmental Pollutions, 115: 253-260.

Zhang Z., Qi H., Ren N., Li Y., Gao D., Kannan K., 2011. Survey of Cyclic and Linear Siloxanes in Sediment from the Songhua River and in Sewage Sludge from Wastewater Treatment Plants, Northeastern China. Archives of Environmental Contamination and Toxicology, 60: 204-211. DOI 10.1007/s00244-010-9619-x.

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